There are two ways you can add articles to folders: you can import them directly from your computer, or you can move a document that’s already in your Mendeley library into that folder.
Direct Import
To add a document that is saved on your computer, open your desired Mendeley folder by clicking on the name of the folder on the left side of the screen. Then, click on the “+ Add New” icon at the top left of the screen, click "File(s) from computer," select the file that you want to add, and click “Open.” Your document will now appear in your folder.
Moving an Existing Document
To move a document that is already in your library into a folder, locate that document in your library by clicking on either “All References” or “Recently Added” on the left side of the screen. When you have found the desired document, single click on it and drag it into the desired folder on the left side of the screen.